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The secret of angry or evil emoticons is in their eyes. Use ` and ´ or ` and ´. Just don't change the characters' order, otherwise your angry emoticon will become friendly and kind (compare: ` ´ - evil eyes, ´ ` - kind eyes). In addition, you can add "wrinkles" # and their stronger forms: メ or ╬; and 凸 (middle finger) and ψ (claws) as an arm. You can also use "snarl" 皿 or 益.